Step 1: Understanding the Concept
A vector in the plane of \(\bar{a}\) and \(\bar{b}\) that is perpendicular to \(\bar{a}\) is parallel to \(\bar{a}\times(\bar{a}\times\bar{b})\).
Step 2: Compute a x b
\(\bar{a}\times\bar{b} = (-3, 3, 3)\).
Step 3: Compute a x (a x b)
\((2, 1, 1)\times(-3, 3, 3) = (0, -9, 9)\), parallel to \((0, -1, 1)\).
Step 4: Match
The vector \(-\hat{j} + \hat{k}\) fits option D.
Final Answer:
The vector is \(-\hat{j} + \hat{k}\).
\[ \boxed{\text{(D) }-\hat{\mathrm{j}}+\hat{\mathrm{k}}} \]