Step 1: Write the surface area of an open cylinder.
For an open cylinder (open at the top), the surface area consists of
\[
\text{Curved Surface Area}+\text{Area of one base}.
\]
Hence,
\[
S=2\pi rh+\pi r^2.
\]
Since the surface area is given and fixed,
\[
2\pi rh+\pi r^2=S.
\]
Therefore,
\[
h=\frac{S-\pi r^2}{2\pi r}.
\]
Step 2: Express the volume in terms of \(r\).
The volume of the cylinder is
\[
V=\pi r^2h.
\]
Substituting the value of \(h\),
\[
V
=
\pi r^2
\left(
\frac{S-\pi r^2}{2\pi r}
\right).
\]
\[
V
=
\frac{r(S-\pi r^2)}{2}.
\]
\[
V
=
\frac{Sr-\pi r^3}{2}.
\]
Step 3: Differentiate and find the critical point.
\[
\frac{dV}{dr}
=
\frac{1}{2}
\left(
S-3\pi r^2
\right).
\]
For maximum volume,
\[
\frac{dV}{dr}=0.
\]
Hence,
\[
S-3\pi r^2=0.
\]
\[
S=3\pi r^2.
\]
Step 4: Find the relation between \(r\) and \(h\).
Using
\[
S=2\pi rh+\pi r^2,
\]
and
\[
S=3\pi r^2,
\]
we get
\[
2\pi rh+\pi r^2=3\pi r^2.
\]
Dividing by \(\pi r\),
\[
2h+r=3r.
\]
\[
2h=2r.
\]
\[
h=r.
\]
Step 5: Verify maximum condition.
\[
\frac{d^2V}{dr^2}
=
-\frac{6\pi r}{2}
=
-3\pi r.
\]
Since \(r\gt 0\),
\[
\frac{d^2V}{dr^2}\lt 0.
\]
Hence the volume is maximum.
Step 6: Final conclusion.
Therefore,
\[
\boxed{r=h}
\]
i.e., the radius is equal to the height of the cylinder.