Concept:
For a matrix
\[
M=\begin{bmatrix}a & b c & d\end{bmatrix},
\]
the adjoint is
\[
\operatorname{adj}M=
\begin{bmatrix}
d & -b
-c & a
\end{bmatrix}.
\]
Step 1: Finding the adjoint of matrix \( A \).
Given,
\[
A=
\begin{bmatrix}
\sec\theta & -\tan\theta
-\tan\theta & \sec\theta
\end{bmatrix}.
\]
Comparing with
\[
\begin{bmatrix}
a & b
c & d
\end{bmatrix},
\]
we get:
\[
a=d=\sec\theta,
\]
and
\[
b=c=-\tan\theta.
\]
Hence,
\[
\operatorname{adj}A=
\begin{bmatrix}
\sec\theta & \tan\theta
\tan\theta & \sec\theta
\end{bmatrix}.
\]
Step 2: Applying the given condition.
We are given:
\[
A+\operatorname{adj}A=4I.
\]
Substituting the matrices:
\[
\begin{bmatrix}
\sec\theta & -\tan\theta
-\tan\theta & \sec\theta
\end{bmatrix}
+
\begin{bmatrix}
\sec\theta & \tan\theta
\tan\theta & \sec\theta
\end{bmatrix}
=
\begin{bmatrix}
4 & 0
0 & 4
\end{bmatrix}.
\]
Adding the matrices:
\[
\begin{bmatrix}
2\sec\theta & 0
0 & 2\sec\theta
\end{bmatrix}
=
\begin{bmatrix}
4 & 0
0 & 4
\end{bmatrix}.
\]
Step 3: Comparing corresponding elements.
Equating diagonal entries:
\[
2\sec\theta=4.
\]
Therefore,
\[
\sec\theta=2.
\]
Thus,
\[
\cos\theta=\frac{1}{2}.
\]
Hence,
\[
\boxed{\theta=\frac{\pi}{3}}.
\]