Concept:
Brachiopods are marine invertebrates having two shells or valves, but their shell symmetry differs from pelecypods.
Step 1: Valve size.
In brachiopods, the two valves are generally unequal in size.
\[
\text{Pedicle valve}\neq \text{brachial valve}
\]
Step 2: Symmetry.
Each valve is bilaterally symmetrical about a median plane, giving equilateral symmetry.
Step 3: Final answer.
Thus, brachiopod valves are unequal in size with equilateral symmetry.
\[
\therefore \text{Correct Answer is (C)}
\]