Step 1: Key Formula:
For \(A = \begin{bmatrix}a & b\\ c & d\end{bmatrix}\), \(\text{adj}\,A = \begin{bmatrix}d & -b\\ -c & a\end{bmatrix}\).
Step 2: Find adj A:
Here \(a = d = \sec\theta\) and \(b = c = -\tan\theta\). So \(\text{adj}\,A = \begin{bmatrix}\sec\theta & \tan\theta\\ \tan\theta & \sec\theta\end{bmatrix}\).
Step 3: Add:
\(A + \text{adj}\,A = \begin{bmatrix}2\sec\theta & 0\\ 0 & 2\sec\theta\end{bmatrix} = 2\sec\theta\, I\).
Set \(2\sec\theta = 4\), so \(\sec\theta = 2\) and \(\cos\theta = \frac12\). With \(\theta\in(0,\frac{\pi}{2})\), \(\theta = \frac{\pi}{3}\).
Final Answer:
The value is \(\theta = \frac{\pi}{3}\), option (C).
\[ \boxed{\frac{\pi}{3}} \]