Step 1: Expand the cube.
We need to expand \( \left( \frac{1}{3} + 3i \right)^3 \). Use the binomial expansion formula:
\[
(a + b)^3 = a^3 + 3a^2b + 3ab^2 + b^3
\]
Here, \( a = \frac{1}{3} \) and \( b = 3i \), so we have:
\[
\left( \frac{1}{3} + 3i \right)^3 = \left( \frac{1}{3} \right)^3 + 3 \left( \frac{1}{3} \right)^2 (3i) + 3 \left( \frac{1}{3} \right) (3i)^2 + (3i)^3
\]
Step 2: Calculate each term.
Now calculate each term:
\[
\left( \frac{1}{3} \right)^3 = \frac{1}{27}
\]
\[
3 \left( \frac{1}{3} \right)^2 (3i) = 3 \times \frac{1}{9} \times 3i = \frac{9i}{9} = i
\]
\[
3 \left( \frac{1}{3} \right) (3i)^2 = 3 \times \frac{1}{3} \times (-9) = -9
\]
\[
(3i)^3 = 27i^3 = 27(-i) = -27i
\]
Step 3: Combine the terms.
Now, combine all the terms:
\[
\left( \frac{1}{3} + 3i \right)^3 = \frac{1}{27} + i - 9 - 27i
\]
Simplify:
\[
\left( \frac{1}{3} + 3i \right)^3 = \frac{1}{27} - 9 + (-26i)
\]
Step 4: Conclusion.
The expression \( \left( \frac{1}{3} + 3i \right)^3 \) in the form \( a + ib \) is:
\[
\boxed{\frac{1}{27} - 9 - 26i}
\]