Concept:
In glass production, different raw materials supply different oxides. Limestone is mainly used to supply calcium oxide.
Step 1: Limestone is calcium carbonate:
\[
CaCO_3
\]
Step 2: During heating, limestone decomposes:
\[
CaCO_3 \rightarrow CaO+CO_2
\]
Step 3: The \(CaO\) produced acts as a stabilizer in soda-lime glass.
Step 4: Soda ash supplies \(Na_2O\), sand supplies \(SiO_2\), and pearl ash supplies \(K_2O\).
Therefore, the most important raw material for supplying \(CaO\) is:
\[
\boxed{\text{Lime stone}}
\]